Transetherification on Polyols by Intra- and Intermolecular Nucleophilic Substitutions

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چکیده

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Transetherification on Polyols by Intra- and Intermolecular Nucleophilic Substitutions

Transetherification on polyols involving intra- and intermolecular nucleophilic substitutions is reported. Di- or trialkoxide formation of propane-1,3-diol or 2-(hydroxymethyl)propane-1,3-diol derivatives by NaH triggers the reaction via oxetanes formation, where the order to add NaH and a polyol significantly influences the yields of products. It was demonstrated that the protective group on t...

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FULL PAPER HBF4 Catalysed Nucleophilic Substitutions of Propargylic Alcohols

The activity of HBF4 (aqueous solution) as a catalyst in propargylation reactions is presented. Diverse types of nucleophiles were employed in order to form new C–O, C–N and C–C bonds in technical acetone, and in air. Good to excellent yields were obtained using low acid loading (typically 1 mol %) under simple reaction conditions and good chemoselectivity.

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ژورنال

عنوان ژورنال: PLoS ONE

سال: 2014

ISSN: 1932-6203

DOI: 10.1371/journal.pone.0091912